Data for: Torsional Force Microscopy of Van der Waals Moires and Atomic Lattices

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Abstract/Contents

Abstract
In a stack of atomically-thin Van der Waals layers, introducing interlayer twist creates a moire superlattice whose period is a function of twist angle. Changes in that twist angle of even hundredths of a degree can dramatically transform the system’s electronic properties. Setting a precise and uniform twist angle for a stack remains difficult, hence determining that twist angle and mapping its spatial variation is very important. Techniques have emerged to do this by imaging the moire, but most of these require sophisticated infrastructure, time-consuming sample preparation beyond stack synthesis, or both. In this work, we show that Torsional Force Microscopy (TFM), a scanning probe technique sensitive to dynamic friction, can reveal surface and shallow subsurface structure of Van der Waals stacks on multiple length scales: the moires formed between bi-layers of graphene and between graphene and hexagonal boron nitride (hBN), and also the atomic crystal lattices of graphene and hBN. In TFM, torsional motion of an AFM cantilever is monitored as the it is actively driven at a torsional resonance while a feedback loop maintains contact at a set force with the surface of a sample. TFM works at room temperature in air, with no need for an electrical bias between the tip and the sample, making it applicable to a wide array of samples. It should enable determination of precise structural information including twist angles and strain in moire superlattices and crystallographic orientation of VdW flakes to support predictable moire heterostructure fabrication.

Description

Type of resource Dataset, text
Date modified December 13, 2023; December 13, 2023
Publication date August 15, 2023

Creators/Contributors

Author Pendharkar, Mihir ORCiD icon https://orcid.org/0000-0003-1857-6131 (unverified)
Author Tran, Steven J.
Author Zaborski Jr., Gregory
Author Finney, Joe
Author Sharpe, Aaron L.
Author Kamat, Rupini V.
Author Kalantre, Sandesh S.
Author Hocking, Marisa
Author Bittner, Nathan ORCiD icon https://orcid.org/0009-0005-7120-0661 (unverified)
Author Watanabe, Kenji
Author Taniguchi, Takashi
Author Pittenger, Bede
Author Newcomb, Christina J.
Author Kastner, Marc A.
Author Mannix, Andrew J.
Author Goldhaber-Gordon, David

Subjects

Subject Torsional Force Microscopy
Subject Moire Superlattices
Subject Van der Waals materials
Genre Data
Genre Tabular data
Genre Data sets
Genre Dataset
Genre Tables (data)

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This work is licensed under a Creative Commons Attribution 4.0 International license (CC BY).

Preferred citation

Preferred citation
Pendharkar, M., Tran, S., Zaborski Jr., G., Finney, J., Sharpe, A., Kamat, R., Kalantre, S., Hocking, M., Bittner, N., Watanabe, K., Taniguchi, T., Pittenger, B., Newcomb, C., Kastner, M., Mannix, A., and Goldhaber-Gordon, D. (2023). Data for: Torsional Force Microscopy of Van der Waals Moires and Atomic Lattices. Stanford Digital Repository. Available at https://purl.stanford.edu/zj475qr8207. https://doi.org/10.25740/zj475qr8207.

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