Electronic and vibrational dynamics of photo-excited A7 structures

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Abstract/Contents

Abstract
The interaction of intense femtosecond laser pulses with matter leads to highly excited transient states far from equilibrium. The dynamics of these excited states relate to many applications from laser machining to energy conversion. Ultrafast optical and x-ray light-scattering has emerged as a powerful experimental method to study material dynamics on the time-scale of atomic and even electronic motion. Here I report results of ultrafast coherent and squeezed phonon scattering experiments in bismuth and antimony. In response to laser-generated coherent phonons, I find dynamics of the coherent A1g vibrational mode greatly dependent on non-thermal electronic band-occupation. And in response to laser generated squeezed phonons, I find anisotropic changes in dynamical forces evidenced by differentiated high wavevector acoustic mode softening. These results advance our understanding of microscopic electron-electron and electron-phonon interactions in transient systems.

Description

Type of resource text
Form electronic; electronic resource; remote
Extent 1 online resource.
Publication date 2015
Issuance monographic
Language English

Creators/Contributors

Associated with Bray, Crystal Christina LaToni
Associated with Stanford University, Department of Applied Physics.
Primary advisor Reis, David A, 1970-
Thesis advisor Reis, David A, 1970-
Thesis advisor Fisher, Ian
Thesis advisor Reed, Evan J
Advisor Fisher, Ian
Advisor Reed, Evan J

Subjects

Genre Theses

Bibliographic information

Statement of responsibility Crystal Christina LaToni Bray.
Note Submitted to the Department of Applied Physics.
Thesis Thesis (Ph.D.)--Stanford University, 2015.
Location electronic resource

Access conditions

Copyright
© 2015 by Crystal Christina Bray
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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