Mechanisms and kinetics of silicon under dynamic compression

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Abstract/Contents

Abstract
This thesis analyzes the dynamic material response of crystalline silicon to laser-driven shock loading. As a shockwave passes through the silicon, it generates a high-pressure, high-temperature environment that causes the material lattice to compress, deform, adopt new high-pressure phases, and eventually enter a melt state. Measuring these responses utilizes an ultra-bright, ultrafast x-ray source capable of capturing the lattice and atomic motions in-situ. The first experiment (Chapter 3) characterizes the loading source, a high-power optical laser at the Matter in Extreme Conditions endstation of the Linac Coherent Light Source. Analysis of the drive system optimized the experimental setup to send steady-pressure, spatially-uniform shockwaves through the silicon. The second experiment (Chapter 4) builds on the results of the first experiment, driving high-pressure (> 20 GPa) shocks through pure crystalline silicon samples. Using a setup configuration that places the x-rays transverse to the optical drive laser beam, this experiment takes simultaneous, ultrafast x-ray diffraction and direct x-ray imaging data of the lattice response. A series of focused spatial and temporal scans determines the kinetics of the elastic, inelastic, and melt waves. Additionally, wide field-of-view x-ray imaging spatially resolves these responses and illuminates an intermediate elastic wave. The third experiment (Chapter 5) analyzes additional data to extract the density of the imaged silicon melt in-situ, a long-standing challenge in the dynamic compression community. It establishes a positive trend between drive pressure and melt density while simultaneously quantifying the change in transformed material volume. A final experiment (Appendix B) examines the photon flux on-target in the Matter in Extreme Conditions endstation. It determines the effect of beamline configuration on the delivered number of x-rays - a critical value for expanding the results of this thesis to new low-transparency and/or high-Z materials.

Description

Type of resource text
Form electronic resource; remote; computer; online resource
Extent 1 online resource.
Place California
Place [Stanford, California]
Publisher [Stanford University]
Copyright date 2019; ©2019
Publication date 2019; 2019
Issuance monographic
Language English

Creators/Contributors

Author Brown, Shaughnessy Brennan
Degree supervisor Cappelli, Mark A. (Mark Antony)
Degree supervisor Mao, Wendy (Wendy Li-wen)
Thesis advisor Cappelli, Mark A. (Mark Antony)
Thesis advisor Mao, Wendy (Wendy Li-wen)
Thesis advisor Nagler, Bob
Degree committee member Nagler, Bob
Associated with Stanford University, Department of Mechanical Engineering.

Subjects

Genre Theses
Genre Text

Bibliographic information

Statement of responsibility Shaughnessy Brennan Brown.
Note Submitted to the Department of Mechanical Engineering.
Thesis Thesis Ph.D. Stanford University 2019.
Location electronic resource

Access conditions

Copyright
© 2019 by Shaughnessy Brennan Brown
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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