Engineering catalyst interfaces for carbon dioxide utilization

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Abstract/Contents

Abstract
CO2 hydrogenation provides the unique opportunity of valorizing this greenhouse gas to a variety of chemicals, and the selectivity towards a specific product relies in first place on the heterogeneous catalysts used to accelerate the rate of the reactions, whose properties are further dictated by their structure. Conventional heterogeneous catalysts consist of multiple elements in their metal and/or oxide form supported on oxide materials, and the interface between the metal(s) and the supporting oxide has been identified as a crucial aspect in achieving reactivity and selectivity beyond what can be obtained with individual components. This dissertation focuses on three types of catalyst interfaces, and the impact of their structure on CO2 hydrogenation reactions. This knowledge acquired during my PhD was utilized to design novel catalyst structures that achieved unprecedented activity and selectivity for CO2 hydrogenation towards valuable products.

Description

Type of resource text
Form electronic resource; remote; computer; online resource
Extent 1 online resource.
Place California
Place [Stanford, California]
Publisher [Stanford University]
Copyright date 2024; ©2024
Publication date 2024; 2024
Issuance monographic
Language English

Creators/Contributors

Author Zhou, Chengshuang
Degree supervisor Cargnello, Matteo
Thesis advisor Cargnello, Matteo
Thesis advisor Bao, Zhenan
Thesis advisor Mai, Danielle
Degree committee member Bao, Zhenan
Degree committee member Mai, Danielle
Associated with Stanford University, School of Engineering
Associated with Stanford University, Department of Chemical Engineering

Subjects

Genre Theses
Genre Text

Bibliographic information

Statement of responsibility Chengshuang Zhou.
Note Submitted to the Department of Chemical Engineering.
Thesis Thesis Ph.D. Stanford University 2024.
Location https://purl.stanford.edu/vv425tq1293

Access conditions

Copyright
© 2024 by Chengshuang Zhou

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