Enhancing the light-matter interaction in graphene

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Abstract/Contents

Abstract
Graphene, a two-dimensional sheet of hexagonally arranged carbon atoms, can absorb 2.3 % of the incident light over a broad range of wavelengths. Whereas the single-layer-absorption is impressive, it is not strong enough for many optoelectronic applications as virtually all the light is transmitted. Moreover, for active devices such as electro-optical modulators and actively controlled thermal emitters, dynamic control over absorption is required as well. We will discuss an electrically-tunable Salisbury screen device configuration that involves placing graphene about a quarter wavelength (λ/4) distance away from a metal back reflector. This design is capable of achieving both increased absorption and active absorption modulation in a single graphene sheet. However, there is an increasing desire to build ultra-compact devices such that the costs of these devices are minimized without compromising on their performance. To satisfy this additional requirement, we combine graphene with metamaterial mirrors that enhance the electric field and hence light-matter interaction within graphene at the mirror surface. We employ Raman spectroscopy to explore the interesting dependence of the electric fields within graphene on the underlying metamaterial mirror dimensions and project the graphene-coated metamaterial mirrors as uniform and tunable SERS (Surface Enhanced Raman Spectroscopy) substrate. As a final step, we perform reflectance measurements on these metamaterial mirrors and establish a direct correlation of these measurements with Raman measurements. We conclude, therefore, that it is possible to predict the strength of our SERS substrate using reflectance measurements solely.

Description

Type of resource text
Form electronic; electronic resource; remote
Extent 1 online resource.
Publication date 2017
Issuance monographic
Language English

Creators/Contributors

Associated with Thareja, Vrinda
Associated with Stanford University, Department of Materials Science and Engineering.
Primary advisor Brongersma, Mark L
Thesis advisor Brongersma, Mark L
Thesis advisor Fan, Shanhui, 1972-
Thesis advisor Harris, J. S. (James Stewart), 1942-
Advisor Fan, Shanhui, 1972-
Advisor Harris, J. S. (James Stewart), 1942-

Subjects

Genre Theses

Bibliographic information

Statement of responsibility Vrinda Thareja.
Note Submitted to the Department of Materials Science and Engineering.
Thesis Thesis (Ph.D.)--Stanford University, 2017.
Location electronic resource

Access conditions

Copyright
© 2017 by Vrinda Thareja
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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