Local thermodynamic probe of correlated electrons in moiré systems

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Abstract/Contents

Abstract
The emergence of "moiré materials", heterostructures formed by twisting and stacking atomically thin layers, has inaugurated a new era for investigating correlated electronic systems. They offer unprecedented tunability over band structure, electronic interactions and topology. In this dissertation, I will present my works on the use of a specialized scanning probe microscope, a scanning single-electron transistor (SET), to locally investigate correlated states in a diverse array of moiré systems. The SET probes the local compressibility and chemical potential of an electronic system with unparalleled resolution, enabling access to the delicate interaction-driven incompressible (insulating) phases and their phase transitions. In this dissertation, I will first summarize instrumentation efforts to set up two different scanning SET systems at Stanford University, which were used to carry out scientific projects described in this dissertation. I will then describe measurements on a selection of representative examples from two distinct classes of moiré materials. In magic-angle twisted bilayer graphene, I explore both the interacting Chern and Hofstadter physics in the high magnetic field regime, as well as the enigmatic correlated insulators found at low magnetic fields. In a semiconductor moiré heterobilayer WSe2/MoSe2, I describe measurements that reveal the coexistence of flat and dispersive moiré bands that leads to intricate competitions between Hofstadter and unconventional charge-ordered states. In a twisted double bilayer WSe2 system, I discuss how the introduction of Γ−valley moiré bands leads to new correlated ground states and charge excitations. Through these measurements, I will demonstrate how the local thermodynamic sensing capabilities of scanning SET synergize with the high tunability of moiré materials in uncovering novel correlated electronic phases.

Description

Type of resource text
Form electronic resource; remote; computer; online resource
Extent 1 online resource.
Place California
Place [Stanford, California]
Publisher [Stanford University]
Copyright date 2023; ©2023
Publication date 2023; 2023
Issuance monographic
Language English

Creators/Contributors

Author Yu, Jiachen
Degree supervisor Feldman, Ben (Benjamin Ezekiel)
Degree supervisor Goldhaber-Gordon, David, 1972-
Thesis advisor Feldman, Ben (Benjamin Ezekiel)
Thesis advisor Goldhaber-Gordon, David, 1972-
Thesis advisor Heinz, Tony F
Degree committee member Heinz, Tony F
Associated with Stanford University, School of Humanities and Sciences
Associated with Stanford University, Department of Applied Physics

Subjects

Genre Theses
Genre Text

Bibliographic information

Statement of responsibility Jiachen Yu.
Note Submitted to the Department of Applied Physics.
Thesis Thesis Ph.D. Stanford University 2023.
Location https://purl.stanford.edu/kr187bt5498

Access conditions

Copyright
© 2023 by Jiachen Yu
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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