Two-pulse x-ray photon correlation spectroscopy at Linac coherent light source

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Abstract/Contents

Abstract
Nearly fully transversely coherent femtosecond x-ray pulses produced by x-ray free electron laser sources opened up the possibilities of direct measurement of atomic scale dynamics of complex systems at their native timescales. One area of particular interest is the investigation of noncrystalline matter such as liquids, glasses, amorphous and disordered systems, and holds the promises of unlocking the mysteries behind the glass transition, liquid-liquid phase transitions, fragile-to-strong transitions, etc. A primary methodology with the potential to extend dynamic light scattering to angstrom and femto- to nanosecond timescale is the so-called two-pulse x-ray photon correlation spectroscopy (XPCS) technique, where the dynamics of the scattering object are imprinted onto the fluctuations of coherent scattering intensity distribution. This dissertation focuses on the instrumentation and methodology of two-pulse XPCS, highlighting the challenges and efforts to establish it as a robust technique at x-ray free electron laser facilities towards measuring ultrafast dynamics in complex matter

Description

Type of resource text
Form electronic resource; remote; computer; online resource
Extent 1 online resource
Place California
Place [Stanford, California]
Publisher [Stanford University]
Copyright date 2020; ©2020
Publication date 2020; 2020
Issuance monographic
Language English

Creators/Contributors

Author Sun, Yanwen
Degree supervisor Bucksbaum, Philip H
Degree supervisor Dunne, Anthony Michael
Thesis advisor Bucksbaum, Philip H
Thesis advisor Dunne, Anthony Michael
Thesis advisor Reis, David A, 1970-
Thesis advisor Sutton, Mark, (Professor of physics)
Degree committee member Reis, David A, 1970-
Degree committee member Sutton, Mark, (Professor of physics)
Associated with Stanford University, Department of Physics.

Subjects

Genre Theses
Genre Text

Bibliographic information

Statement of responsibility Yanwen Sun
Note Submitted to the Department of Physics
Thesis Thesis Ph.D. Stanford University 2020
Location electronic resource

Access conditions

Copyright
© 2020 by Yanwen Sun
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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