Study of nanoscale magnetization dynamics and reversal following ultrafast optical excitation by resonant X-ray diffraction

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Abstract/Contents

Abstract
In 1996, femtosecond (fs) optical laser pulse was first discovered by as one of the novel methods to quench the magnetization[1]. While the fs optical laser pulses typically induces demagnetization, they are also discovered to be able to cause all-optical switching (AOS) of magnetic domains in the transition metal-rare earth (TM-RE) alloy GdFeCo[2, 3, 4, 5, 6]. This phenomenon not only opened door for fascinating non-equilibrium magnetism research but also brought forth the possibility of optical control of magnetism in future magnetic recording technologies. In this thesis, we take an microscopic approach to study the optically-induced magnetization dynamics by utilizing x-ray diffraction technique. We are able to address some important physics questions and technological relevancy regarding the phenomenon. The technological potential of AOS has recently increased with the discovery of the same effect in other materials, including RE-free magnetic multilayers[7, 8]. However, to be technologically competitive for the bit density requirement of future storage device, AOS must further restrict its optically-switched magnetic areas to sizes well below the diffraction limit. By deploying gold plasmonic antenna structure on the surface of ferrimagnetic TbFeCo alloy, we demonstrate reproducible and robust all-optical switching of magnetic domains of 53 nm size. The nanoscale magnetic reversal is imaged both around and beneath plasmonic antennas using x-ray resonant holographic imaging technique. Furthermore, our results also demonstrate the importance of the sample chemical nanostructure on the magnetic switching. The microscopic dynamics of magnetization following an fs optical excitation is also studied in the similar material GdFeCo. Based on theoretical predictions[9, 10], we searched for magnetic solitons generated from spin wave condensation in the far-from-equilibrium condition induced by fs optical excitation. By studying the resonant x-ray diffraction pattern, we present evidence of such soliton feature formation in magnetization dynamics experimentally. We also relate the microscopic magnetization picture to the bulk magnetization response of the sample.

Description

Type of resource text
Form electronic; electronic resource; remote
Extent 1 online resource.
Publication date 2017
Issuance monographic
Language English

Creators/Contributors

Associated with Liu, Tianmin
Associated with Stanford University, Department of Physics.
Primary advisor Stöhr, Joachim
Thesis advisor Stöhr, Joachim
Thesis advisor Kasevich, Mark A
Thesis advisor Reis, David A, 1970-
Advisor Kasevich, Mark A
Advisor Reis, David A, 1970-

Subjects

Genre Theses

Bibliographic information

Statement of responsibility TianMin Liu.
Note Submitted to the Department of Physics.
Thesis Thesis (Ph.D.)--Stanford University, 2017.
Location electronic resource

Access conditions

Copyright
© 2017 by TianMin Liu
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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