Thermal phenomena in nanostructured materials & devices
Abstract/Contents
- Abstract
- Nanostructuring leads to unique material properties and combinations of properties not naturally available in bulk materials. The study of these properties is critical to improving the device performance and reliability for a range of applications including electronics, thermoelectrics, and nanophotonics. This work focuses on efforts to push the thermal conductivity of nanostructured materials to the extremes: the thermal conductivity of carbon nanotubes (CNT) and nanotube-based materials can exceed that of metals, while the introduction of nanoscale boundaries (e.g. nanoscale pores in silicon nanowires) yields extremely low thermal conductivity materials. Furthermore, this nanostructuring also leads to unique combinations of properties. Porous silicon nanowires are a step towards the desired electron-crystal, phonon-glass combination ideal for thermoelectric applications, while thermally-conductive, mechanically-compliant carbon nanotube films for promising for electronics packaging. This work first explores how the high axial thermal conductivity of carbon nanotubes can be leveraged effectively in thin film and composites through detailed understanding of the phonon transport and measurements of CNT-based films. This work then investigates how nanostructuring silicon significantly reduces the thermal conductivity through enhanced boundary scattering and the possibility of phononic crystal effects. Specifically, measurements of individual, porous silicon nanowires and arrays of silicon nanowires show significant reduction in the thermal conductivity compared to bulk silicon. A detailed model for reduced thermal conductivity due to phonon boundary scattering is developed in conjunction with measurements. Finally, this work also examines how the composition and annealing conditions impact both thermal transport and photoluminescence in silicon-rich silicon nitride films.
Description
Alternative title | Thermal phenomena in nanostructured materials and devices |
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Type of resource | text |
Form | electronic; electronic resource; remote |
Extent | 1 online resource. |
Publication date | 2012 |
Issuance | monographic |
Language | English |
Creators/Contributors
Associated with | Marconnet, Amy Marie |
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Associated with | Stanford University, Department of Mechanical Engineering |
Primary advisor | Goodson, Kenneth E, 1967- |
Thesis advisor | Goodson, Kenneth E, 1967- |
Thesis advisor | Vuckovic, Jelena |
Thesis advisor | Zheng, Xiaolin, 1978- |
Advisor | Vuckovic, Jelena |
Advisor | Zheng, Xiaolin, 1978- |
Subjects
Genre | Theses |
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Bibliographic information
Statement of responsibility | Amy Marie Marconnet. |
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Note | Submitted to the Department of Mechanical Engineering. |
Thesis | Thesis (Ph.D.)--Stanford University, 2012. |
Location | electronic resource |
Access conditions
- Copyright
- © 2012 by Amy Marie Marconnet
- License
- This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).
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