Evolution of the charge density wave state in the rare-earth tritellurides under uniaxial stress and disorder

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Abstract/Contents

Abstract
Materials with strong electron correlations often exhibit a complex interplay between competing or coexisting ordered phases, such as charge order, magnetism, and superconductivity. Model systems which isolate just one of these components, however, can provide a practical path for navigating this complexity. This dissertation provides detailed studies of the behavior of the rare-earth tritellurides (RTe3 where R=Y, La-Nd, Sm, Gd-Tm) a candidate model system under two different perturbations, namely uniaxial stress and disorder. First, however, I present the results of analytical and numerical modeling of heat flow in measurements of the AC elastocaloric effect (AC-ECE), a new experimental tool that I use to investigate the title compounds. My work demonstrates that the details of the frequency-dependent sensitivity in AC-ECE measurements are highly nontrivial, and I present both intuitive explanations of these effects as well as a quantitative match with experiment. I apply the AC-ECE technique to explore the effects of in-plane uniaxial stress on the CDW transitions in both ErTe3 and TmTe3. A combination of AC-ECE measurements, together with in-plane and out-of-plane elastoresistivity measurements, clearly detects changes in the critical temperatures, transport anisotropy, and thermodynamic quantities as a function of strain. Finally, I describe the transport, thermodynamic, and scattering characteristics of single crystals of PdxErTe3, in which neutral Pd atoms intercalated between the Te bilayers act as a weak random potential. This work has established RTe3 as a model system for studying the interplay of unidirectional CDW formation, in-plane uniaxial stress, disorder, and superconductivity. Further investigation of the inter-relation of these effects could have direct bearing on a range of other material systems of current interest

Description

Type of resource text
Form electronic resource; remote; computer; online resource
Extent 1 online resource
Place California
Place [Stanford, California]
Publisher [Stanford University]
Copyright date 2020; ©2020
Publication date 2020; 2020
Issuance monographic
Language English

Creators/Contributors

Author Straquadine, Joshua Alan Wolfe
Degree supervisor Fisher, Ian R. (Ian Randal)
Thesis advisor Fisher, Ian R. (Ian Randal)
Thesis advisor Hwang, Harold Yoonsung, 1970-
Thesis advisor Kivelson, Steven
Degree committee member Hwang, Harold Yoonsung, 1970-
Degree committee member Kivelson, Steven
Associated with Stanford University, Department of Applied Physics.

Subjects

Genre Theses
Genre Text

Bibliographic information

Statement of responsibility Joshua Alan Wolfe Straquadine
Note Submitted to the Department of Applied Physics
Thesis Thesis Ph.D. Stanford University 2020
Location electronic resource

Access conditions

Copyright
© 2020 by Joshua Alan Wolfe Straquadine
License
This work is licensed under a Creative Commons Attribution Non Commercial 3.0 Unported license (CC BY-NC).

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