Effects of optical and environmental parameters on angle-resolved photoemission from materials

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Abstract/Contents

Abstract
Studies in condensed matter physics have led to the discovery of a profusion of materials with interesting quantum properties, such as superconductors and topological insulators. The wide variety of material systems demands a wide variety of experimental techniques. I focus on two techniques: angle-resolved photoemission spectroscopy (ARPES), which measures electronic band structure in the energy and momentum domains; and time-resolved ARPES, which probes out-of-equilibrium phenomena by extending ARPES to the time domain. There are many parameters which can affect measurements of quantum materials. I show how varying nonlinear crystal thickness in an ultrafast laser setup allows for fine-tunable time and energy resolution in time-resolved photoemission. Achieving a high degree of control over resolutions is critical for enabling new experiments. I also investigate how Bi2Se3 surfaces change to bismuth upon exposure to air, potentially affecting results of surface-sensitive measurements in atmosphere. High control and understanding of temporal, spectroscopic, and sample composition properties, as well as the optical and environmental parameters which control them, are essential to performing successful experiments on quantum materials.

Description

Type of resource text
Form electronic resource; remote; computer; online resource
Extent 1 online resource.
Place California
Place [Stanford, California]
Publisher [Stanford University]
Copyright date 2021; ©2021
Publication date 2021; 2021
Issuance monographic
Language English

Creators/Contributors

Author Gauthier, Alexandre Vance
Degree supervisor Shen, Zhi-Xun
Thesis advisor Shen, Zhi-Xun
Thesis advisor Devereaux, Thomas Peter, 1964-
Thesis advisor Heinz, Tony F
Degree committee member Devereaux, Thomas Peter, 1964-
Degree committee member Heinz, Tony F
Associated with Stanford University, Department of Applied Physics

Subjects

Genre Theses
Genre Text

Bibliographic information

Statement of responsibility Alexandre Gauthier.
Note Submitted to the Department of Applied Physics.
Thesis Thesis Ph.D. Stanford University 2021.
Location https://purl.stanford.edu/cv948sj9645

Access conditions

Copyright
© 2021 by Alexandre Vance Gauthier
License
This work is licensed under a Creative Commons Attribution 3.0 Unported license (CC BY).

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